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李远志:博士、二级教授、博士生导师,2003年6月在南京大学化学化工学院获博士学位,2004年4月至2006年8月在日本理化学研究所前沿研究系统任研究员,自2006年9月起任武汉理工大学教授,湖北省自然科学基金创新团队学术带头人,国家科学技术奖会评专家,J. Am. Chem. Soc.,Angew. Chem. Int. Ed.等30多种国际重要期刊审稿人。近几年来,先后承担国家重大研究计划项目课题、国家自然科学基金项目、教育部重大项目、湖北省自然科学基金创新团队项目等10余项,在纳微结构氧化物及其复合物的合成、催化性能及隔热性能等方面,开展了系统深入的研究工作,取得了一批创新性研究成果,研发了系列光谱响应宽、催化效率高、稳定性好的空气污染物净化和太阳能-化学能转化新材料,以及隔热性能优异的绝热材料。先后Adv. Mater.,Adv. Eng. Mater.,J. Am. Chem. Soc., Adv. Funct. Mater., ACS Catal., Chem. Mater.,Appl. Catal. B., J. Mater. Chem.(A), Nanoscale, ACS Appl. Mater. Interfaces, Environ. Sci. Technol.等在多种国际重要期刊发表SCI论文80余篇,论文被它引3000余次;获国际专利1项、国家发明专利授权6项和日本专利2项;多次在相关国际会议上作邀请报告;获湖北省自然科学二等奖(排名第一, 2017)。
主要研究方向:
1、光催化、热催化、光热协同催化纳微结构空气污染物净化材料。
2、热催化及光热协同催化CO2转化、制氢及太阳能-化学能转化材料。
3、纳微结构绝热、节能材料。
近几年主持的主要项目:
1. 基于介孔CeO2限域纳米VIII簇金属的新金属载体作用和表面等离子体效应的太阳光驱动催化干法甲烷重整, 国家自然科学基金项目,2017.1-2020.12。
2. 全太阳光谱驱动纳米结构OMS-2催化净化挥发性有机污染物,国家自然科学基金项目,2015.1-2018.12。
3. 半导体氧化物纳米晶的晶面、缺陷调控及其对光热协同催化净化VOCs性能的影响,国家自然科学基金项目,2013.1-2016.12。
4. TiO2基纳米光催化材料及器件的制备与性能优化,国家重大研究计划项目课题, 2009.1-2013.12。
5. 新型纳孔建筑保温防火材料的开发及产业化,湖北省科技厅科技支撑项目,2014.1-2015.12。
6. 基于光催化和多相催化耦合的汽车尾气净化材料的应用基础研究, 湖北省创新群体项目, 2011.1-2012.12。
7. 三维有序大孔/介孔半导体薄膜的微结构调控及其在污染治理中的应用,教育部重大项目,2009.1-2011.12。
部分代表性论文
[1] H. Huang, M. Y. Mao, Y. Z. Li* (通讯作者), J. L. Bai, Q. Zhang, Y. Yang, M. Zeng, X. J. Zhao, Solar-light-driven CO2 reduction by CH4 on silica cluster modified Ni nanocrystals with high solar-to-fuel efficiency and excellent durability, Adv. Energy Mater. 2018, 201702472.
[2] C. Y. Zhou, L. Cheng, Y. Z. Li*, M. Zeng, Y. Yang, J. C. Wu, X. J. Zhao, Novel photoactivation promotes catalytic abatement of CO on CuO mesoporous nanosheets with full solar spectrum illumination, Appl. Catal. B 2018, 225, 314–323.
[3] L. Lan, Z. K. Shi, Q. Zhang, Y. Z. Li*, Y. Yang, S. W. Wu, X. J. Zhao, Defects lead to a massive enhancement in UV-Vis-IR driven thermocatalytic activity of Co3O4 mesoporous nanorods, J. Mater. Chem. A, 2018, DOI: 10.1039/C8TA01362D.
[4] Y. Yang, Y. Z. Li*, M. Zeng, M. Y. Mao, L. Lan, H. H. Liu, J. Chen, X. J. Zhao, UV–vis-infrared light-driven photothermocatalytic abatement of CO on Cu doped ramsdellite MnO2 nanosheets enhanced by a photoactivation effect, Appl. Catal. B 2018, 224, 751–760.
[5] J. Chen, Y. Z. Li*, S. M. Fang, Y. Yang, X. J. Zhao, UV–Vis-infrared light-driven thermocatalytic abatement of benzene on Fe doped OMS-2 nanorods enhanced by a novel photoactivation, Chem. Eng. J. 2018, 332, 205–215.
[6] M. Zeng, Y. Z. Li*, F. Liu, Y. Yang, M. Y. Mao, X. J. Zhao, Cu doped OL-1 nanoflower: A UV-vis-infrared light-driven catalyst for gas-phase environmental purification with very high efficiency, Appl. Catal. B 2017, 200, 521–529.
[7] L. Lan, Y. Z. Li*, M. Zeng, M. Y. Mao, L. Ren, Y. Yang, H. H. Liu, L. Yun, X.J. Zhao, Efficient UV–vis-infrared light-driven catalytic abatement of benzeneon amorphous manganese oxide supported on anatase TiO2nanosheet with dominant {001} facets promoted by aphotothermocatalytic synergetic effect, Appl. Catal. B, 2017, 203, 494–504.
[8] Y. Yang, Y. Z. Li,* M. Y. Mao, M. Zeng, X. J. Zhao, UV−Visible−Infrared Light Driven Thermocatalysis for Environmental Purification on Ramsdellite MnO2 Hollow Spheres Considerably Promoted by a Novel Photoactivation, ACS Appl. Mater. Interfaces 2017, 9, 2350−2357.
[9] S. M. Fang, Y. Z. Li*, Y. Yang, J. Chen, H. H. Liu, X. J. Zhao, Mg doped OMS-2 nanorod: A highly efficient catalyst for purification of volatile organic compounds with full solar spectrum irradiation, Environ. Sci.: Nano, 2017, 4, 1798–1807.
[10] F. Liu, M. Zeng, Y. Z. Li*, Y. Yang, M. Y. Mao, X. J. Zhao, UV-Vis-Infrared Light Driven Thermocatalytic Activity of Octahedral Layered Birnessite Nanoflowers Enhanced by a Novel Photoactivation, Adv. Funct. Mater. 2016, 26, 4518-4526.
[12] M. Y. Mao, H. Q. Lv, Y. Z. Li*, Y. Yang, M. Zeng, X. J. Zhao, Metal Support Interaction in Pt Nanoparticles Partially Confined in the Mesopores of Microsized Mesoporous CeO2 for Highly Efficient Purification of Volatile Organic Compounds, ACS Catal. 2016, 6, 418−427.
[13] L. Ren, Y. Z. Li*, J. T. Hou, J. L. Bai, M. Y. Mao, M. Zeng, X. J. Zhao, N. Li, The Pivotal Effect of the Interaction between Reactant and Anatase TiO2 Nanosheets with Exposed {001} Facets on Photocatalysis for the Photocatalytic Purification of VOCs,Appl. Catal. B 2016, 181, 625-634.
[14] H. H. Liu, Y. Z. Li*, Y. Yang, M. Y. Mao, M. Zeng, L. Lan, L. Yun, X. J. Zhao, Highly efficient UV-Vis-infrared catalytic purification of benzene on CeMnxOy/TiO2nanocomposite, caused by its high thermocatalytic activity and strong absorption in the full solar spectrum region, J. Mater. Chem. A, 2016, 4, 9890-9899.
[15] M. Zeng, Y. Z. Li*, M. Y. Mao, J. L. Bai, L. Ren, X. J. Zhao, Synergetic Effect between Photocatalysis on TiO2 and Thermocatalysis on CeO2 for Gas-Phase Oxidation of Benzene on TiO2/CeO2 Nanocomposites, ACS Catal. 2015, 5, 3278−3286.
[16] M. Y. Mao, Y. Z. Li*, J. T. Hou, M. Zeng, X. J. Zhao, Extremely efficient full solar spectrum light driven thermocatalyticactivity for the oxidation of VOCs on OMS-2 nanorod catalyst, Appl. Catal. B 2015, 174, 496–503.
[17] Y. Ma, Y. Z. Li*, M. Y. Mao, J. T. Hou, M. Zeng, X. J. Zhao, Synergetic effect between photocatalysis on TiO2 and solar light-driven thermocatalysis on MnOx for benzene purification on MnOx/TiO2 nanocomposites, J. Mater. Chem. A, 2015, 3, 5509–5516.
[18] J. T. Hou, Y. Z. Li*, M. Y. Mao, Y. Z. Yue, G. N. Greaves, X. J. Zhao, Full solar spectrum light driven thermocatalysis with extremely high efficiency on nanostructured Ce ion substituted OMS-2 catalyst for VOCs Purification, Nanoscale, 2015, 7, 2633–2640.
[19] J. T. Hou, Y. Z. Li*, M. Y. Mao, X. J. Zhao, Y. Z. Yue, The effect of Ce ion substituted OMS-2 nanostructure in catalytic activity for benzene oxidation, Nanoscale, 2014, 6, 15048–15058.
[20] L. Ren, Y. Z. Li*, J. T. Hou, X. J. Zhao, X. C. Pan, Preparation and Enhanced Photocatalytic Activity of TiO2 Nanocrystals with Internal Pores, ACS Appl. Mater. Interfaces 2014, 6, 1608−1615.
[21] J. T. Hou , Y. Z. Li*, M. Y. Mao , L. Ren , X. J. Zhao, Tremendous Effect of the Morphology of Birnessite-Type Manganese Oxide Nanostructures on Catalytic Activity, ACS Appl. Mater. Interfaces, 2014, 6, 14981–14987.
[22] J. T. Hou, L. L. Liu, Y. Z. Li*, M. Y. Mao, H. Q. Lv, X. J. Zhao, Tuning the K+Concentration in the Tunnel of OMS-2 Nanorods Leads to a Significant Enhancement of the Catalytic Activity for Benzene Oxidation, Environ. Sci. Technol. 2013, 47, 13730-13736.
[23] J. T. Hou, Y. Z. Li*, L. L. Liu, L. Ren, X. J. Zhao, Effect of giant oxygen vacancy defects on the catalytic oxidation of OMS-2 nanorods, J. Mater. Chem. A 2013, 1, 6736–6741.
[24] W. Q. Shi, Y. Z. Li*, J. T. Hou, H. Q. Lv, X. J. Zhao, P. F. Fang, F. Zheng, S. J. Wang, Densely Populated Mesopores in Microcuboid CeO2 Crystal Leads to a Significant Enhancement of Catalytic Activity,J. Mater. Chem. A 2013, 1, 728-734.
[25] L. Ren, T. T. Tian, Y. Z. Li*, J. G. Huang, X. J. Zhao, High-Performance UV Photodetection of Unique ZnO Nanowires from Zinc Carbonate Hydroxide Nanobelts, ACS Appl. Mater. Interfaces 2013, 5, 5861–5867.
[27] S. F. Jin, Y. Z. Li*, H. Xie, X. Chen, T. T. Tian, X. J. Zhao, Highly Selective Photocatalytic and Sensing Properties of 2D-Ordered Dome films of Nano Titania and Nano Ag2+ doped Titania, J. Mater. Chem. 2012, 22, 1469-1476.
[28] W. Xie, Y. Z. Li*, W.Q. Shi, L. Zhao, X. J. Zhao, P. F. Fang, F. Zheng, S. J. Wang,Novel effect of significant enhancement of gas-phase photocatalytic efficiency for nano ZnO, Chem. Eng. J. 2012, 213, 218–224.
[29] M. Kong, Y. Z. Li*, X. Chen, T. T. Tian, P. F. Fang, F. Zheng, X. J. Zhao, Tuning the Relative Concentration Ratio of Bulk Defects to Surface Defects in TiO2 Nano Crystal Leads to High Efficient Photocatalytic Efficiency, J. Am. Chem. Soc. 2011, 133, 16414–16417.
[30] W. Sun, Y. Z. Li*, W. Q. Shi, X. J. Zhao, P. F. Fang, Formation of AgI/TiO2Nanocomposite Leads to Excellent Thermochromic Reversibility and Photostability, J. Mater. Chem. 2011, 21, 9263-9270.
[31] Q. Yue, Y. Z. Li*, M. Kong, J. C. Huang, X. J. Zhao, J.Liu, R. E Williford,Ultralow Density, Hollow Silica Foams Through Interfacial Reaction and Their Exceptional Properties for Environmental and Energy Applications, J. Mater. Chem. 2011, 21, 12041-12046.
联系方式:
1、Tel:
2、E-mail:liyuanzhi66@hotmail.com; liyuanzhi@whut.edu.cn;
3、工作地址(实验室):武汉理工大学硅酸盐建筑材料国家重点实验室500-3室。
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